CCL:G: "gen" keyword for ONIOM



 Sent to CCL by: "Marius Retegan" [marius.s.retegan!^!gmail.com]
 I think that warning that you are getting is self explanatory, you
 have to define a basis set for your hydrogen atoms. For example if you
 have cluster of Si and H, try using something like this at the end of
 your input:
 Si
 6-31G*
 ****
 H
 3-21G*
 ****
 I don't know believe that geom=connectivity has any connection with you error.
 Marius
 On 7/31/07, Gonzalo Jim nez-Os s gonzalo.jimenez]![unirioja.es
 <owner-chemistry,+,ccl.net> wrote:
 >
 > Sent to CCL by: "Gonzalo  Jim  nez-Os  s"
 [gonzalo.jimenez-x-unirioja.es]
 > Dear Nihan,
 >
 > I frequently get similar messages using ONIOM in G03, but I think that it
 is not striclty related to the use of the "gen" keyword. Note that
 employing the AM1 method generates a lot of warnings, what is a bit
 disturbing...Nevertheless, the failure in the SCF step (over 129 cycles) is more
 related with some inconsistency within the QM part. Try to add the keyword
 "geom=connectivity" to the input and/or to prepare a better starting
 structure in order to facilitate the generation of a more realiable initial
 guess. I hope it helps,
 >
 > Regards,
 >
 > ========================================================
 > Gonzalo Jimnez-Oss
 > Complejo Cientfico Tecnolgico
 > Departamento de Qumica. Universidad de La Rioja
 > Grupo de Sntesis Qumica de la Rioja, U.A.-C.S.I.C.
 > C/ Madre de Dios, 51. E-26006 Logroo (La Rioja). Spain
 > Tfn. +34-941-299630      Fax  +34-941-299621
 > gonzalo.jimenez\a/unirioja.es
 > http://www.unirioja.es/cu/gojimeo
 > ========================================================
 >
 > ------------------------
 > Sent to CCL by: "Nihan  Aldis" [naldis ~~ gmail.com]
 > Dear CCLers,
 > When I use gen keyword in Oniom calculation on a Silicon cluster, I have
 some problems.  This is part of my input:
 > RunGauss
 > %chk=Si353Gen2
 > %nproc=1
 > %mem=1000MB
 > p opt oniom(b3lyp/Gen:am1/sparse) gfinput iop(6/7=3)
 >
 > gen
 >
 > 0 1 0 1 0 1
 >  Si               0    1.724600   -4.250418    1.968610 H
 >  Si               0    3.751190   -3.034175    1.924736 L H      1
 >  Si               0    5.662891   -4.357333    1.929145 L
 >  Si               0    6.231758   -5.525771    3.838685 L
 >  Si               0    8.593935   -5.661679    3.806473 L
 >  Si               0    9.324290   -4.582704    5.732750 L
 >  Si               0   11.401024   -3.435620    5.647742 L
 >  Si               0   11.390783   -1.944169    3.792553 L
 >  Si               0    9.600614   -0.392726    3.864778 L
 >  Si               0    9.613309    0.972654    1.922365 L
 >  Si               0    9.567945   -0.388159    0.000714 L
 >  Si               0    9.613275    0.961448   -1.928825 L
 >  Si               0    9.600508   -0.415218   -3.863267 L
 >  Si               0   11.390636   -1.966275   -3.782136 L
 > ......................
 > ........................
 >  H                0    0.000606   14.105707    3.098136 L
 >  H                0    1.190799   15.481702   -0.037854 L
 >  H                0   -1.202043   15.474212   -0.037516 L
 >
 > 40 50 107 140 152 160 0
 > 6-31G*
 > ****
 > 1 41 51 76 93 94 108 131 0
 > 3-21G*
 > ****
 > 132 141 153 161 169 175 185 0
 > 3-21G*
 > ****
 >
 > When it ran, I got the following error in the output:
 >
 >  Warning!  H  atom  172 has  1 valence electrons but only   0 basis
 functions.
 >  This is less than a minimal basis set!
 >  Warning!  H  atom  176 has  1 valence electrons but only   0 basis
 functions.
 >  This is less than a minimal basis set!
 >  Warning!  H  atom  182 has  1 valence electrons but only   0 basis
 functions.
 >  This is less than a minimal basis set!
 >  Warning!  H  atom  186 has  1 valence electrons but only   0 basis
 functions.
 >  This is less than a minimal basis set!
 >  Warning!  H  atom  195 has  1 valence electrons but only   0 basis
 functions.
 >  This is less than a minimal basis set!
 >
 >  IExCor= 402 DFT=T Ex=B+HF Corr=LYP ExCW=0 ScaHFX=  0.200000
 >  ScaDFX=  0.800000  0.720000  1.000000  0.810000
 >  IRadAn=      0 IRanWt=     -1 IRanGd=            0 ICorTp=0
 >  NAtoms=  334 NActive=   41 NUniq=   41 SFac= 1.00D+00 NAtFMM=   60 Big=F
 >  Leave Link  301 at Fri Jul 27 15:31:01 2007, MaxMem=  131072000 cpu:
 0.0
 >  (Enter /home/g03/l302.exe)
 > ........................
 > ...........................
 >
 >  >>>>>>>>>> Convergence criterion not met.
 >  SCF Done:  E(RB+HF-LYP) =  -6064.80456753     A.U. after  129 cycles
 >              Convg  =    0.8803D-04             -V/T =  2.0032
 >              S**2   =   0.0000
 >  KE= 6.045687912820D+03 PE=-2.555956789915D+04 EE= 7.901465986937D+03
 >  Convergence failure -- run terminated.
 >  Error termination via Lnk1e in /home/g03/l502.exe at Sat Jul 28 13:38:31
 2007.
 >  Job cpu time:  0 days 22 hours  6 minutes 44.1 seconds.
 >  File lengths (MBytes):  RWF=    669 Int=      0 D2E=      0 Chk=    391
 Scr=      1
 >
 > What can I do to use both the ONIOM and the gen keyword? Is there anything
 to add my input?
 > Thank you
 > Nihan Aldishttp://www.ccl.net/cgi-bin/ccl/send_ccl_messagehttp-:-//www.ccl.net/chemistry/sub_unsub.shtmlhttp-:-//www.ccl.net/spammers.txt--
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