CCL:G: Pre-optimization



Dear Joseph,

you can try out our recently developed HF-3c method. It is based on a HF/minimal(small) basis set calculation and therefore fast. Three atom pair-wise correction terms are applied to correct the HF energy with respect to London dispersion interactions (D3 scheme), basis set superposition error (gCP scheme), and short-ranged basis set incompleteness effects. More details can be found in the publication:

   J. Comput. Chem. 34, 1672–1685 (2013)

The HF-3c method yields good geometries for standard organic molecules, supramolecules and proteins.

HF-3c is implemented in the free ORCA software suite. You can simply invoke it by the keyword ! HF-3c.
As you cannot use our method with G09 you would have to switch to a different program but it is probably worth trying.

Cheers,
Rebecca

--

Rebecca Sure, M.Sc. (rebecca.sure=-=thch.uni-bonn.de)
Mulliken Center for Theoretical Chemistry
Institut für Physikalische und Theoretische Chemie
Universität Bonn, Beringstr. 4, D-53115 Bonn



On 06/20/2013 02:54 AM, Joseph Takayama sjtakayama*|*gmail.com wrote:
Sent to CCL by: "Joseph  Takayama" [sjtakayama-*-gmail.com]
 Hi Everyone,
 I'm trying to optimize some transition state structure with B3LYP/6-31G*.
 I'd like to do pre-optimization in order to shorten the calculation time and
 see if my initial structure works.
 I might need to do some try & error, so I'd like to shorten the calculation
 time as much as possible for pre-optimization.
 Among the following options, which do you think is acceptable?
 1. Change method to HF, AM1 or PM3.
 2. Change basis function to 3-21G* or to STO-3G.
 3. Add SCF=(conver=4)
 4. Add opt=loose.
 5. Is there any other way to reduce calculation time??
 I'm using Gaussian 09 and my main targets are organic molecule just contains
 H,C,N,O atoms and inorganic complex contains one transition metal.E-mail to
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